Neutron capture cross-section measurements with TC-Pn in KUR for some nuclides targeted for decommissioning

Nakamura, Shoji; Endo, Shunsuke; Kimura, Atsushi; Shibahara, Yuji*

KURNS Progress Report 2022, P. 73, 2023/07

The present study is concerned with the neutron capture cross-sections that contribute to the evaluation of the amount of radionuclides possessing problems in decommissioning. In this study, Sc, Cu, Zn, Ag, In and W were selected among the objective nuclides, and their thermal-neutron capture cross-sections were measured using TC-Pn equipment of the KUR of the Institute for Integrated Radiation and Nuclear Science, Kyoto University. High purity metal samples were prepared. A gold-aluminum ally wire, cobalt and molybdenum foils were used to monitor the neutron flux at the irradiation position of TC-Pn. The flux monitors and metal samples were irradiated for 1 hour at 1-MW operation of the KUR. After irradiation, the irradiation capsule was opened, samples and flux monitors were enclosed in a vinyl bag one by one, and then rays emitted from the samples and monitors were measured with a high-purity Ge detector. The thermal-neutron flux component was derived with the reaction rates of flux monitors (Au, Co and Mo) on the basis of Westcott's convention, and found to be (5.920.10)10 n/cm/sec at the irradiation position. The measured reaction rate for each metal sample divided by the evaluated thermal-neutron capture cross-section should give the same value of the thermal-neutron flux component if the cross section is suitable. This time, we found that the cross sections of Sc and Zn were consistent with the evaluated one, but those of other nuclides were inconsistent with their evaluated ones; that is, it turned out that their thermal-neutron capture cross-sections should be modified.

Simultaneous determination of zircon crystallisation age and temperature; Common thermal evolution of mafic magmatic enclaves and host granites in the Kurobegawa granite, central Japan

Yuguchi, Takashi*; Yamazaki, Hayato*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Suzuki, Satoshi*; Ogita, Yasuhiro; Sando, Kazusa*; Imura, Takumi*; Ono, Takeshi*

Journal of Asian Earth Sciences, 226, p.105075_1 - 105075_9, 2022/04

https://doi.org/10.1016/j.jseaes.2021.105075

Simultaneous determination of the U-Pb age of zircon and concentration of titanium in a single analysis spot, using inductively coupled plasma mass spectrometry with laser ablation sample introduction, produces paired age and temperature data of zircon crystallisation, potentially revealing time-temperature () histories for evolved magma. The Kurobegawa granite, central Japan, contains abundant mafic magmatic enclaves (MMEs). We applied this method to evaluate MMEs and their host (enclosing) granites. Cooling behaviour common to both MMEs and host rocks was found between 1.5 and 0.5 Ma. Rapid cooling from the zircon crystallisation temperature to the closure temperature of biotite K-Ar system was within 1 million year. Combining the obtained paths of MMEs and host rocks with petrological information can provide insights into magma chamber processes. This suggests that MME flotation, migration, and spread through the magma chamber ceased at 1.5-0.5 Ma, indicating the emplacement age of the Kurobegawa granitic pluton, as no large-scale reheating episodes have occurred since then.

spectrometry of terrestrial gamma rays using portable germanium detectors in area of 80 km radius around the Fukushima Daiichi Nuclear Power Plant

Mikami, Satoshi; Tanaka, Hiroyuki*; Okuda, Naotoshi*; Sakamoto, Ryuichi*; Ochi, Kotaro; Uno, Kiichiro*; Matsuda, Norihiro; Saito, Kimiaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(4), p.159 - 178, 2021/12

https://doi.org/10.3327/taesj.J20.010

In order to know the background radiation level where the area affected by the Fukushima Daiichi Nuclear Power Plant accident in 2011, terrestrial gamma rays had been measured by using portable germanium detectors repeatedly from 2013 through 2019, at 370 locations within 80 km radius area centered on the Fukushima Daiichi Nuclear Power Plant. Radioactive concentrations of Uranium 238, Thorium 232, Potassium 40 and kerma rates in air due to terrestrial gamma rays were obtained at those locations based on the method of ICRU report 53. Averaged concentrations of U, Th and K were 18.8, 22.7, 428 Bq/kg, respectively, and kerma rate in air over the area was found to be 0.0402 Gy/h. The obtained kerma rates in air were compared to those reported in literatures. It was confirmed that the data were correlated with each other, and were agreed within the range of their uncertainty. This is because the kerma rate in air due to terrestrial gamma rays is depend on geology. The similar trend to previous findings was observed that the kerma rate in air at locations geologically classified as Mesozoic era, Granite and Rhyolite were statistically significantly higher than the others.

Evaluation of decreasing trend in air dose rate and ecological half-life within an 80 km range from Fukushima Dai-ichi Nuclear Power Plant, using car-borne survey data measured by KURAMA systems up to 2018

Ando, Masaki; Sasaki, Miyuki; Saito, Kimiaki

Journal of Nuclear Science and Technology, 57(12), p.1319 - 1330, 2020/12

https://doi.org/10.1080/00223131.2020.1789008

Air dose rates measured by car-borne surveys within 80 km range of Fukushima Dai-ichi Nuclear Power Plant using KURAMA systems from 2011 up to 2018 were analyzed, and decreasing trends and ecological half-life were evaluated. The decreasing speed of air dose rates became 0.08 over a period of seven years, indicating a much more rapid decrease than estimated by the physical decay of radiocesium (0.3). The fast components of the ecological half-lives evaluated in entire the evacuation order area were about 2 to 3 y, and were considerably larger than those outside the evacuation order area (0.4 to 0.5 y). To model the acceleration in the decrease of air dose rates observed in evacuation order areas, we modified the bi-exponential curve formula of ecological half-life and introduced the two-group model. The fast decreasing components of the ecological half-life evaluated using the two-group model after 2013 were 0.5 to 1 y, and were much shorter than those up to 2013, at 2 to 3 y.

External dose evaluation based on detailed air dose rate measurements in living environments

Sato, Tetsuro*; Ando, Masaki; Sato, Masako*; Saito, Kimiaki

Journal of Environmental Radioactivity, 210, p.105973_1 - 105973_7, 2019/12

https://doi.org/10.1016/j.jenvrad.2019.05.005

A method was devised for estimation of external doses of Fukushima residents expected to return to their homes after evacuation orders are lifted. 211 residents expected to return to six towns and villages were surveyed in FY 2014, FY 2015, and FY2016. Interviewing returning residents about their expected life patterns after returning, air dose rate were measured along the reported personal trails representing their patterns of movement in daily life. Excluding 15 residents from whose homes we were unable to take air dose rate measurements, the maximum external effective dose and the average external effective dose were estimated respectively as 4.9 mSv/y and 0.86 mSv/y. Although the mean values and dispersion of external effective doses differ depending on the evacuation level, for 93.3% of all residents, the estimated external effective doses were less than 2 mSv/y. The average exposure dose at home accounts for 66.8% of the annual exposure dose.

Decreasing trend of ambient dose equivalent rates over a wide area in eastern Japan until 2016 evaluated by car-borne surveys using KURAMA systems

Ando, Masaki; Mikami, Satoshi; Tsuda, Shuichi; Yoshida, Tadayoshi; Matsuda, Norihiro; Saito, Kimiaki

Journal of Environmental Radioactivity, 192, p.385 - 398, 2018/12

https://doi.org/10.1016/j.jenvrad.2018.07.009

Car-borne surveys using KURAMA systems have been conducted over a wide area in eastern Japan since 2011. The measurement data collected until 2016 was analyzed, and decreasing trend of the dose rates in regions within 80 km of Fukushima Dai-ichi Nuclear Power Plant were examined. The averaged dose rates tended to decrease considerably with respect to the physical decay of radiocaesium, and the ecological half-lives of the fast and slow decay components were estimated. The decrease of the dose rate in the forest was slower than its decrease in other regions, and the decrease of the dose rate in urban area was the fastest. The decrease in the dose rates obtained via the car-borne survey was larger than that obtained on flat ground with few disturbances using survey meters approximately 1.5 y after the accident; hereafter, the decrease in the dose rates obtained via the car-borne survey was same as the latter measurement.

Measurement of ambient dose equivalent rates by walk survey around Fukushima Dai-ichi Nuclear Power Plant using KURAMA-II until 2016

Ando, Masaki; Yamamoto, Hideaki*; Kanno, Takashi*; Saito, Kimiaki

Journal of Environmental Radioactivity, 190-191, p.111 - 121, 2018/10

https://doi.org/10.1016/j.jenvrad.2018.04.025

Ambient dose equivalent rates in various environments related to human lives were measured by walk surveys using the KURAMA-II systems from 2013 to 2016 around the Fukushima Dai-ichi Nuclear Power Plant. The dose rate of the locations where the walk survey was performed decreased to about 38% of its initial value in the 42 months, which was beyond that attributable to the physical decay. The air dose rates decreased depending on the level of the evacuation areas, and the decrease was slightly larger in populated areas where humans are active. The comparison of walk survey data with car-borne survey data indicated that the air dose rate varies largely even within a 100 m square area. The dose rates measured by the walk surveys were estimated to be medial of those along roads and those of undisturbed flat ground. The air dose rates measured by the walk surveys decreased quickly compared with the air dose rate from the flat ground measurement.

Evaluation of ambient dose equivalent rates owing to natural radioactive nuclides in eastern Japan by car-borne surveys using KURAMA-II

Ando, Masaki; Matsuda, Norihiro; Saito, Kimiaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 16(2), p.63 - 80, 2017/05

https://doi.org/10.3327/taesj.J16.023

In order to discriminate the contribution of radioactive cesium due to the Fukushima Dai-ichi Nuclear Power Plant accident to the air dose rates measured by the car-borne surveys, natural background radiation was evaluated for eastern Japan area as the municipality averaged values. The window count method for distinction between natural and artificial radioactive nuclides was applied to the car-borne surveys using the KURAMA-II. Distribution of the evaluated natural background radiation showed geological feature, and it was found that the radiations measured along paved roads were reflecting the distribution of terrestrial -rays. The effect of the radioactive cesium as of 2014 for the municipalities designated as the Intensive Contamination Survey Area was beyond the uncertainty of the natural background radiation. That for the other municipalities, however, was found to be almost negligible.

Measurements of americium isotopes by activation method at KURRI-Linac

Nakamura, Shoji; Terada, Kazushi; Takahashi, Yoshiyuki*; Sano, Tadafumi*; Hori, Junichi*

KURRI Progress Report 2015, P. 69, 2016/08

http://www.rri.kyoto-u.ac.jp/PUB/report/PR/ProgRep2015/PR2015.pdf#page=78

Neutron capture cross section measurements has been conducted for Minor Actinides (MAs) under the research project entitled by "Research and development for Accuracy Improvement of neutron nuclear data on Minor ACtinides (AIMAC)". The present work selected two americium isotopes, Am and Am, were selected, and measurements were carried out by an activation method with neutron sources at KURRI-Linac. It was found that the neutron flux at the target positon was of the order of 10 (n/cms). The reaction rates of Am and Am were obtained by - and -ray measurements of the irradiated Am samples.

Study on decreasing trend of air dose rates observed in Fukushima Prefecture and neighboring prefectures

Ando, Masaki; Kanno, Takashi; Saito, Kimiaki

JAEA-Technology 2015-060, 40 Pages, 2016/03

JAEA-Technology-2015-060.pdf:50.1MB

The ratios of air dose rate averaged in prefecture-wise measured by car borne surveys in wide area has been performed by with the use of the KURAMA and KURAMA-II systems were investigated. The changes in air dose rate from the first (June 2011) car borne survey to the fourth (September 2012) and seventh (November 2013) car borne surveys in Fukushima Prefecture was similar to those in Tochigi Prefecture, and the ratio in Miyagi Prefecture showed quicker decay than those in the other prefectures in the groups of less than 0.5Sv/h. Distribution maps of the ratios of air dose rate obtained in 100m mesh wise in Fukushima, Tochigi and Miyagi prefectures showed that the ratios (i.e. decreasing rates) were depending on the area or road. Further, decreasing in the air dose rate was quicker than the physical decay in the big cities where population is big and the traffic is huge.